The kinetics of an irreversible catalytic reaction on a substrate of arbitrary dimension is examined. In the limit of infinitesimal reaction rate (reaction-controlled limit), we solve the dimer-dimer surface reaction model (or voter model) exactly in arbitrary dimension D. The density of reactive interfaces is found to exhibit a power-law decay for D<2 and a slow logarithmic decay in two dimensions. We discuss the relevance of these results for the monomer-monomer surface reaction model.
%0 Journal Article
%1 Frachebourg1996Exact
%A Frachebourg, L.
%A Krapivsky, P. L.
%D 1996
%I American Physical Society
%J Physical Review E
%K kinetics, voter-model lattice-models
%N 4
%P R3009--R3012
%R 10.1103/physreve.53.r3009
%T Exact results for kinetics of catalytic reactions
%U http://dx.doi.org/10.1103/physreve.53.r3009
%V 53
%X The kinetics of an irreversible catalytic reaction on a substrate of arbitrary dimension is examined. In the limit of infinitesimal reaction rate (reaction-controlled limit), we solve the dimer-dimer surface reaction model (or voter model) exactly in arbitrary dimension D. The density of reactive interfaces is found to exhibit a power-law decay for D<2 and a slow logarithmic decay in two dimensions. We discuss the relevance of these results for the monomer-monomer surface reaction model.
@article{Frachebourg1996Exact,
abstract = {{The kinetics of an irreversible catalytic reaction on a substrate of arbitrary dimension is examined. In the limit of infinitesimal reaction rate (reaction-controlled limit), we solve the dimer-dimer surface reaction model (or voter model) exactly in arbitrary dimension D. The density of reactive interfaces is found to exhibit a power-law decay for D<2 and a slow logarithmic decay in two dimensions. We discuss the relevance of these results for the monomer-monomer surface reaction model.}},
added-at = {2019-06-10T14:53:09.000+0200},
author = {Frachebourg, L. and Krapivsky, P. L.},
biburl = {https://www.bibsonomy.org/bibtex/2eec8579082d7854e53fcea2860e832b9/nonancourt},
citeulike-article-id = {6088419},
citeulike-linkout-0 = {http://dx.doi.org/10.1103/physreve.53.r3009},
citeulike-linkout-1 = {http://link.aps.org/abstract/PRE/v53/i4/pR3009\_1},
citeulike-linkout-2 = {http://link.aps.org/pdf/PRE/v53/i4/pR3009\_1},
doi = {10.1103/physreve.53.r3009},
interhash = {8fd2a77e135e2b9fb57e7615d0210bfc},
intrahash = {eec8579082d7854e53fcea2860e832b9},
journal = {Physical Review E},
keywords = {kinetics, voter-model lattice-models},
month = apr,
number = 4,
pages = {R3009--R3012},
posted-at = {2014-01-17 11:58:32},
priority = {2},
publisher = {American Physical Society},
timestamp = {2019-08-01T15:36:09.000+0200},
title = {{Exact results for kinetics of catalytic reactions}},
url = {http://dx.doi.org/10.1103/physreve.53.r3009},
volume = 53,
year = 1996
}